Highly efficient photovoltaic energy storage hybrid system based on ultrathin carbon electrodes designed for a portable and flexible power source
Integrated perovskite solar capacitor (IPSC) systems are the new paradigm for power generation and storage. Herein, a novel configuration and combination of materials for an IPSC, theoretically affording a maximized areal capacitance of 2.35 mF cm−2 and exceeding a 25% overall photo-chemical-electri...
Main Authors: | , , , , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
Elsevier Ltd
2019
|
Subjects: | |
Online Access: | http://umpir.ump.edu.my/id/eprint/25320/ http://umpir.ump.edu.my/id/eprint/25320/ http://umpir.ump.edu.my/id/eprint/25320/ http://umpir.ump.edu.my/id/eprint/25320/1/Highly%20efficient%20photovoltaic%20energy%20storage%20hybrid%20system%20based%20.pdf |
id |
ump-25320 |
---|---|
recordtype |
eprints |
spelling |
ump-253202019-10-25T02:49:15Z http://umpir.ump.edu.my/id/eprint/25320/ Highly efficient photovoltaic energy storage hybrid system based on ultrathin carbon electrodes designed for a portable and flexible power source Farhadi, Bita Marriam, Ifra Yang, Shengyuan Zhang, Hui Tebyetekerwa, Mike Zhu, Meifang Ramakrishna, Seeram Rajan, Jose Zabihi, Fatemeh TK Electrical engineering. Electronics Nuclear engineering TP Chemical technology Integrated perovskite solar capacitor (IPSC) systems are the new paradigm for power generation and storage. Herein, a novel configuration and combination of materials for an IPSC, theoretically affording a maximized areal capacitance of 2.35 mF cm−2 and exceeding a 25% overall photo-chemical-electricity energy conversion efficiency is reported. A ∼1 μm solid-state photocapacitor is suggested based on a CH3NH3PbI3 photoactive layer, inorganic buffer junctions, an ultrathin nanocarbon border and top electrodes. For the first time, bulk and interfacial imperfections in the perovskite layer are reckoned in simulation, realizing the recombination rate to 14-order of magnitude higher than that in the perfect perovskite structure. The simulation considers the band gap energy, the valance and conduction bands, carrier mobility and carrier density of every individual layer of the designed IPSC. Overall, the results for the areal capacitance, output voltage and photocharging efficiency under various illumination conditions, frequencies and dielectric materials show that the performance of the perovskite power pack is mildly susceptible to external and internal triggers. This ultrathin and sturdy architecture, shows promise for use in self-powered portable and wearable personal devices. Elsevier Ltd 2019-05-15 Article PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/25320/1/Highly%20efficient%20photovoltaic%20energy%20storage%20hybrid%20system%20based%20.pdf Farhadi, Bita and Marriam, Ifra and Yang, Shengyuan and Zhang, Hui and Tebyetekerwa, Mike and Zhu, Meifang and Ramakrishna, Seeram and Rajan, Jose and Zabihi, Fatemeh (2019) Highly efficient photovoltaic energy storage hybrid system based on ultrathin carbon electrodes designed for a portable and flexible power source. Journal of Power Sources, 422. pp. 196-207. ISSN 0378-7753 (Print), 1873-2755 (Online) https://doi.org/10.1016/j.jpowsour.2019.02.091 https://doi.org/10.1016/j.jpowsour.2019.02.091 |
repository_type |
Digital Repository |
institution_category |
Local University |
institution |
Universiti Malaysia Pahang |
building |
UMP Institutional Repository |
collection |
Online Access |
language |
English |
topic |
TK Electrical engineering. Electronics Nuclear engineering TP Chemical technology |
spellingShingle |
TK Electrical engineering. Electronics Nuclear engineering TP Chemical technology Farhadi, Bita Marriam, Ifra Yang, Shengyuan Zhang, Hui Tebyetekerwa, Mike Zhu, Meifang Ramakrishna, Seeram Rajan, Jose Zabihi, Fatemeh Highly efficient photovoltaic energy storage hybrid system based on ultrathin carbon electrodes designed for a portable and flexible power source |
description |
Integrated perovskite solar capacitor (IPSC) systems are the new paradigm for power generation and storage. Herein, a novel configuration and combination of materials for an IPSC, theoretically affording a maximized areal capacitance of 2.35 mF cm−2 and exceeding a 25% overall photo-chemical-electricity energy conversion efficiency is reported. A ∼1 μm solid-state photocapacitor is suggested based on a CH3NH3PbI3 photoactive layer, inorganic buffer junctions, an ultrathin nanocarbon border and top electrodes. For the first time, bulk and interfacial imperfections in the perovskite layer are reckoned in simulation, realizing the recombination rate to 14-order of magnitude higher than that in the perfect perovskite structure. The simulation considers the band gap energy, the valance and conduction bands, carrier mobility and carrier density of every individual layer of the designed IPSC. Overall, the results for the areal capacitance, output voltage and photocharging efficiency under various illumination conditions, frequencies and dielectric materials show that the performance of the perovskite power pack is mildly susceptible to external and internal triggers. This ultrathin and sturdy architecture, shows promise for use in self-powered portable and wearable personal devices. |
format |
Article |
author |
Farhadi, Bita Marriam, Ifra Yang, Shengyuan Zhang, Hui Tebyetekerwa, Mike Zhu, Meifang Ramakrishna, Seeram Rajan, Jose Zabihi, Fatemeh |
author_facet |
Farhadi, Bita Marriam, Ifra Yang, Shengyuan Zhang, Hui Tebyetekerwa, Mike Zhu, Meifang Ramakrishna, Seeram Rajan, Jose Zabihi, Fatemeh |
author_sort |
Farhadi, Bita |
title |
Highly efficient photovoltaic energy storage hybrid system based on ultrathin carbon electrodes designed for a portable and flexible power source |
title_short |
Highly efficient photovoltaic energy storage hybrid system based on ultrathin carbon electrodes designed for a portable and flexible power source |
title_full |
Highly efficient photovoltaic energy storage hybrid system based on ultrathin carbon electrodes designed for a portable and flexible power source |
title_fullStr |
Highly efficient photovoltaic energy storage hybrid system based on ultrathin carbon electrodes designed for a portable and flexible power source |
title_full_unstemmed |
Highly efficient photovoltaic energy storage hybrid system based on ultrathin carbon electrodes designed for a portable and flexible power source |
title_sort |
highly efficient photovoltaic energy storage hybrid system based on ultrathin carbon electrodes designed for a portable and flexible power source |
publisher |
Elsevier Ltd |
publishDate |
2019 |
url |
http://umpir.ump.edu.my/id/eprint/25320/ http://umpir.ump.edu.my/id/eprint/25320/ http://umpir.ump.edu.my/id/eprint/25320/ http://umpir.ump.edu.my/id/eprint/25320/1/Highly%20efficient%20photovoltaic%20energy%20storage%20hybrid%20system%20based%20.pdf |
first_indexed |
2023-09-18T22:38:49Z |
last_indexed |
2023-09-18T22:38:49Z |
_version_ |
1777416776993210368 |