Methane production over Ni Supported F-Sba-15: Different amount ff Ni loadings

Formation of bulky wastes of carbon dioxide (CO2) from burning of fossil fuels had impacted to the earth’s environmental issues. The CO2 gases trapped in the ozone layer and thus mitigate the climate change through the greenhouse gases (GHGs) effect. Numerous attentions have been drawn towards recyc...

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Main Authors:	S. N., Bukhari, Setiabudi, H. D., Nurul Aini, Razali, Triwahyono, S., Jalil, A. A.
Format:	Conference or Workshop Item
Language:	English
Published:	2018
Subjects:	TP Chemical technology
Online Access:	http://umpir.ump.edu.my/id/eprint/23720/ http://umpir.ump.edu.my/id/eprint/23720/1/Methane%20production%20over%20Ni%20Supported%20F-Sba-15-%20Different%20amount%20ff%20Ni%20loadings.pdf

id	ump-23720
recordtype	eprints
spelling	ump-237202019-01-10T03:31:18Z http://umpir.ump.edu.my/id/eprint/23720/ Methane production over Ni Supported F-Sba-15: Different amount ff Ni loadings S. N., Bukhari Setiabudi, H. D. Nurul Aini, Razali Triwahyono, S. Jalil, A. A. TP Chemical technology Formation of bulky wastes of carbon dioxide (CO2) from burning of fossil fuels had impacted to the earth’s environmental issues. The CO2 gases trapped in the ozone layer and thus mitigate the climate change through the greenhouse gases (GHGs) effect. Numerous attentions have been drawn towards recycling and transformation of CO2 gases into more valuable products via CO2 methanation by using variety of supported metal catalysts [1–2]. For the choice of support, mesoporous material type of support such as SBA-15 is preferred due to its favorable textural properties with higher surface area (600-1,000 m2/g), larger pore size diameter (5-30 nm), higher thermal and hydrothermal stability as well as highly uniform-arranged mesopores. Nickel (Ni) is selected as type of metal due to its low price and easily available [3]. However, if the carbon deposition and metal sintering occurred over metal-based support, it may rapidly trigger the deactivation of catalyst due to weaker interaction between metal and support [4], and thus resulted to a lower catalytic performance towards methane production. Therefore, this study highlighted on the modification structure of SBA-15 support into fibrous type (F-SBA-15) in order to produce higher accessibility of metal to be dispersed into it due to the formation of higher surface area and wide pore diameter, in agreement with Firmansyah et al. [5]. In addition, different amount of Ni loadings (1, 3, 5, and 10 wt.%) onto F-SBA-15 support for methane production were also controlled. Their physical properties were characterized using XRD, BET, and FTIR. In-situ FTIR adsorbed pyrrole analysis revealed the presence of basic sites originated in the catalysts. 2018 Conference or Workshop Item PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/23720/1/Methane%20production%20over%20Ni%20Supported%20F-Sba-15-%20Different%20amount%20ff%20Ni%20loadings.pdf S. N., Bukhari and Setiabudi, H. D. and Nurul Aini, Razali and Triwahyono, S. and Jalil, A. A. (2018) Methane production over Ni Supported F-Sba-15: Different amount ff Ni loadings. In: 4th International Conference Of Chemical Engineering And Industrial Biotechnology (ICCEIB 2018), 1-2 Aug 2018 , Seri Pacific Hotel, Kuala Lumpur. .
repository_type	Digital Repository
institution_category	Local University
institution	Universiti Malaysia Pahang
building	UMP Institutional Repository
collection	Online Access
language	English
topic	TP Chemical technology
spellingShingle	TP Chemical technology S. N., Bukhari Setiabudi, H. D. Nurul Aini, Razali Triwahyono, S. Jalil, A. A. Methane production over Ni Supported F-Sba-15: Different amount ff Ni loadings
description	Formation of bulky wastes of carbon dioxide (CO2) from burning of fossil fuels had impacted to the earth’s environmental issues. The CO2 gases trapped in the ozone layer and thus mitigate the climate change through the greenhouse gases (GHGs) effect. Numerous attentions have been drawn towards recycling and transformation of CO2 gases into more valuable products via CO2 methanation by using variety of supported metal catalysts [1–2]. For the choice of support, mesoporous material type of support such as SBA-15 is preferred due to its favorable textural properties with higher surface area (600-1,000 m2/g), larger pore size diameter (5-30 nm), higher thermal and hydrothermal stability as well as highly uniform-arranged mesopores. Nickel (Ni) is selected as type of metal due to its low price and easily available [3]. However, if the carbon deposition and metal sintering occurred over metal-based support, it may rapidly trigger the deactivation of catalyst due to weaker interaction between metal and support [4], and thus resulted to a lower catalytic performance towards methane production. Therefore, this study highlighted on the modification structure of SBA-15 support into fibrous type (F-SBA-15) in order to produce higher accessibility of metal to be dispersed into it due to the formation of higher surface area and wide pore diameter, in agreement with Firmansyah et al. [5]. In addition, different amount of Ni loadings (1, 3, 5, and 10 wt.%) onto F-SBA-15 support for methane production were also controlled. Their physical properties were characterized using XRD, BET, and FTIR. In-situ FTIR adsorbed pyrrole analysis revealed the presence of basic sites originated in the catalysts.
format	Conference or Workshop Item
author	S. N., Bukhari Setiabudi, H. D. Nurul Aini, Razali Triwahyono, S. Jalil, A. A.
author_facet	S. N., Bukhari Setiabudi, H. D. Nurul Aini, Razali Triwahyono, S. Jalil, A. A.
author_sort	S. N., Bukhari
title	Methane production over Ni Supported F-Sba-15: Different amount ff Ni loadings
title_short	Methane production over Ni Supported F-Sba-15: Different amount ff Ni loadings
title_full	Methane production over Ni Supported F-Sba-15: Different amount ff Ni loadings
title_fullStr	Methane production over Ni Supported F-Sba-15: Different amount ff Ni loadings
title_full_unstemmed	Methane production over Ni Supported F-Sba-15: Different amount ff Ni loadings
title_sort	methane production over ni supported f-sba-15: different amount ff ni loadings
publishDate	2018
url	http://umpir.ump.edu.my/id/eprint/23720/ http://umpir.ump.edu.my/id/eprint/23720/1/Methane%20production%20over%20Ni%20Supported%20F-Sba-15-%20Different%20amount%20ff%20Ni%20loadings.pdf
first_indexed	2023-09-18T22:35:39Z
last_indexed	2023-09-18T22:35:39Z
_version_	1777416577590755328

Methane production over Ni Supported F-Sba-15: Different amount ff Ni loadings

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