Enhanced Catalytic Performance Of Ni/Sba-15 Towards Co2 Methanation Via P123-Assisted Method

This study focused on the enhancement of catalytic performance of Ni/SBA-15 towards CO2 methanation via P123(PEG-PPG-PEG triblock copolymer)-assisted impregnation method. The pysical and chemical properties of the catalysts were characterized using XRD, BET and FTIR, meanwhile the catalytic performa...

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Main Authors:	Syahida Nasuha, Bukhari, A. H. K., Owgi, N. Aini, Razali, Vo, Dai-Viet N., Setiabudi, H. D.
Format:	Conference or Workshop Item
Language:	English
Published:	2017
Subjects:	TP Chemical technology
Online Access:	http://umpir.ump.edu.my/id/eprint/19325/ http://umpir.ump.edu.my/id/eprint/19325/1/Enhanced%20Catalytic%20Performance%20Of%20Ni-Sba-15%20Towards%20Co2%20Methanation%20Via%20P123-Assisted%20Method.pdf

id	ump-19325
recordtype	eprints
spelling	ump-193252018-10-18T06:12:08Z http://umpir.ump.edu.my/id/eprint/19325/ Enhanced Catalytic Performance Of Ni/Sba-15 Towards Co2 Methanation Via P123-Assisted Method Syahida Nasuha, Bukhari A. H. K., Owgi N. Aini, Razali Vo, Dai-Viet N. Setiabudi, H. D. TP Chemical technology This study focused on the enhancement of catalytic performance of Ni/SBA-15 towards CO2 methanation via P123(PEG-PPG-PEG triblock copolymer)-assisted impregnation method. The pysical and chemical properties of the catalysts were characterized using XRD, BET and FTIR, meanwhile the catalytic performance of catalysts towards CO2 methanation were evaluated using stainless steel fixed bed reactor. The presence of coke on the surface of catalysts was characterized using TGA analysis. XRD and BET results revealed that the dispersion of Ni particles on the surface of SBA-15 were improved with P123 (Ni/SBA-15(P123)) as compared to without P123 (Ni/SBA-15). FTIR analysis revealed that P123 enhanced the formation of metal-support interaction (Si-O-Ni) through the substitution of O‒H with O‒Ni. Ni/SBA-15(P123) exhibited higher activity, better stability and less carbon formation owing to its smaller metal particles, stronger metal-support interaction and more homogenous metal dispersion, which altered the properties of catalyst towards an excellent catalytic performance. This study provides new perspective on the beneficial effect of P123- assisted impregnation method in the enhancement of catalytic performance of Ni/SBA-15 towards CO2 methanation. 2017 Conference or Workshop Item PeerReviewed application/pdf en http://umpir.ump.edu.my/id/eprint/19325/1/Enhanced%20Catalytic%20Performance%20Of%20Ni-Sba-15%20Towards%20Co2%20Methanation%20Via%20P123-Assisted%20Method.pdf Syahida Nasuha, Bukhari and A. H. K., Owgi and N. Aini, Razali and Vo, Dai-Viet N. and Setiabudi, H. D. (2017) Enhanced Catalytic Performance Of Ni/Sba-15 Towards Co2 Methanation Via P123-Assisted Method. In: The 3rd International Conference on Green Chemical Engineering and Technology (3rd GCET), 7-8 November 2017 , Melaka, Malaysia. p. 1.. (Unpublished)
repository_type	Digital Repository
institution_category	Local University
institution	Universiti Malaysia Pahang
building	UMP Institutional Repository
collection	Online Access
language	English
topic	TP Chemical technology
spellingShingle	TP Chemical technology Syahida Nasuha, Bukhari A. H. K., Owgi N. Aini, Razali Vo, Dai-Viet N. Setiabudi, H. D. Enhanced Catalytic Performance Of Ni/Sba-15 Towards Co2 Methanation Via P123-Assisted Method
description	This study focused on the enhancement of catalytic performance of Ni/SBA-15 towards CO2 methanation via P123(PEG-PPG-PEG triblock copolymer)-assisted impregnation method. The pysical and chemical properties of the catalysts were characterized using XRD, BET and FTIR, meanwhile the catalytic performance of catalysts towards CO2 methanation were evaluated using stainless steel fixed bed reactor. The presence of coke on the surface of catalysts was characterized using TGA analysis. XRD and BET results revealed that the dispersion of Ni particles on the surface of SBA-15 were improved with P123 (Ni/SBA-15(P123)) as compared to without P123 (Ni/SBA-15). FTIR analysis revealed that P123 enhanced the formation of metal-support interaction (Si-O-Ni) through the substitution of O‒H with O‒Ni. Ni/SBA-15(P123) exhibited higher activity, better stability and less carbon formation owing to its smaller metal particles, stronger metal-support interaction and more homogenous metal dispersion, which altered the properties of catalyst towards an excellent catalytic performance. This study provides new perspective on the beneficial effect of P123- assisted impregnation method in the enhancement of catalytic performance of Ni/SBA-15 towards CO2 methanation.
format	Conference or Workshop Item
author	Syahida Nasuha, Bukhari A. H. K., Owgi N. Aini, Razali Vo, Dai-Viet N. Setiabudi, H. D.
author_facet	Syahida Nasuha, Bukhari A. H. K., Owgi N. Aini, Razali Vo, Dai-Viet N. Setiabudi, H. D.
author_sort	Syahida Nasuha, Bukhari
title	Enhanced Catalytic Performance Of Ni/Sba-15 Towards Co2 Methanation Via P123-Assisted Method
title_short	Enhanced Catalytic Performance Of Ni/Sba-15 Towards Co2 Methanation Via P123-Assisted Method
title_full	Enhanced Catalytic Performance Of Ni/Sba-15 Towards Co2 Methanation Via P123-Assisted Method
title_fullStr	Enhanced Catalytic Performance Of Ni/Sba-15 Towards Co2 Methanation Via P123-Assisted Method
title_full_unstemmed	Enhanced Catalytic Performance Of Ni/Sba-15 Towards Co2 Methanation Via P123-Assisted Method
title_sort	enhanced catalytic performance of ni/sba-15 towards co2 methanation via p123-assisted method
publishDate	2017
url	http://umpir.ump.edu.my/id/eprint/19325/ http://umpir.ump.edu.my/id/eprint/19325/1/Enhanced%20Catalytic%20Performance%20Of%20Ni-Sba-15%20Towards%20Co2%20Methanation%20Via%20P123-Assisted%20Method.pdf
first_indexed	2023-09-18T22:27:43Z
last_indexed	2023-09-18T22:27:43Z
_version_	1777416078891155456

Enhanced Catalytic Performance Of Ni/Sba-15 Towards Co2 Methanation Via P123-Assisted Method

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